France is out of the European Championship, and it was Kylian Mbappe that missed the penalty kick in the shootout.
Switzerland eliminated the World Cup champions 5-4 in the shootout after a 3-3 draw on Monday (Tuesday AEST) in the round of 16.
Switzerland goalkeeper Yann Sommer, who left the team during the group stage to be with his wife for the birth of their daughter, made the decisive safe on the 10th penalty after the previous nine had all been successful.
The Swiss will next play Spain in the quarter-finals in St Petersburg on Friday (Saturday AEST).
Haris Seferovic put Switzerland in the lead with a header in the 15th minute as France struggled to work itself into the game. But that all changed early in the second half when the Swiss were awarded a penalty.
France goalkeeper Hugo Lloris, the team's captain, made the save on Ricardo Rodríguez in the 55th minute and woke up the French. Karim Benzema scored once in the 57th, and again in the 59th to give France the lead.
Paul Pogba made it 3-1 in the 75th with a stunning right-foot shot from 20 metres and it looked like the game was out of reach for the Swiss. But just as quickly as France had taken over the game, they let it go again.
Seferovic scored another header in the 81st minute and Gavranović made it 3-3 with only seconds remaining.
SPAIN 5, CROATIA 3 AFTER EXTRA TIME
Spain first gifted Croatia a bizarre own-goal, then threw away a late 3-1 lead. Alvaro Morata made sure it didn't matter in the end.
Morata and Mikel Oyarzabal scored in extra time Monday (Tuesday AEST) to give Spain a 5-3 win over Croatia and a place in the European Championship quarterfinals after a wildly entertaining see-saw match at Parken Stadium.
It was the second-highest scoring game in the history of the European Championship, trailing only Yugoslavia's 5-4 win over France in the opening game of the inaugural tournament in 1960.
And it had nearly as many momentum shifts as goals.
After Croatia midfielder Mario Pasalic equalized in injury time to cap an improbable late comeback, the much-maligned Morata scored what proved the winner in the 100th minute.
The Spain striker controlled a cross with one deft touch and then sent a rising shot past goalkeeper Dominik Livakovic for his second goal of the tournament.
Oyarzabal doubled the lead three minutes later, receiving a pass in the middle of the area and holding off a defender before scoring.
Morata had received a torrent of online abuse — including death threats — after a string of misses during the group stage. But his fierce finish from a tight angle proved decisive on Monday.
"I don't think there's any coach in the world who wouldn't admire a player like Morata," Spain coach Luis Enrique said. "He dominates in the air, he scores goals, he is physically powerful. He is a striker we should really value."
Spain had been knocked out in the round of 16 in its previous two tournaments but netted five goals for a second straight game after a slow start with two draws. The Spanish will play either France or Switzerland in the quarterfinals on Friday in St. Petersburg.
Croatia netted three goals for a second straight game but fell well short of replicating its feat of reaching the World Cup final in 2018.
"At the start of extra time we had them on the ropes but we failed to score from two good chances," Croatia captain Luka Modric said. "Then the game turned around and we didn't have the strength to come back."
Not for a second time, anyway.
Spain had led 3-1 in the 85th minute but Mislav Orsic pulled one back after a goalmouth scramble and Pasalic equalized with a header in injury time.
Spain had dominated the first 20 minutes but goalkeeper Unai Simon was at fault for his team's early deficit after a massive blunder when he failed to control a long back pass. The ball bounced over Simon's foot and trickled into the net behind him.
"We know that's football and that those things happen," Spain captain Sergio Busquets said. "The most important thing is to pick yourself up and show a strong mentality. And I think both Unai and the whole team did that today."
Spain quickly recovered and Pablo Sarabia equalized in the 38th. Right back Cesar Azpilicueta then made it 2-1 with a header in the 57th and Ferran Torres doubled the lead when he finished off a quick counterattack with a low shot past Livakovic in the 77th.
It looked like Spain was heading for an easy win before Croatia fought back.
"Boy, we had to suffer there," Azpilicueta said. "It wasn't great to be scored against twice late in normal time, but we were the better team in extra time and we deserve to go through."
Croatia's late surge allowed both Morata and Simon to redeem themselves.
The goalkeeper made a crucial save to deny Andrej Kramaric at the start of extra time, then got up and punched the air in celebration.
"I think that when we missed that chance at 3-3 in extra time, that was the determining factor," Croatia coach Zlatko Dalic said. "I think if we had scored a goal it would have been completely different."
Simon also made a big stop at 3-2 when he got down quickly to make a one-handed save on Josko Gvardiol's shot from just outside the box.
"We have complete confidence in (Simon)," Busquets said. "He was unlucky with that own-goal but Unai has a very laid-back mentality. He's very ambitious at the same time and I think he showed that with his reaction, and with the saves he made."
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